Born to Hall Cary and Carol Campbell Thomas in East Cleveland, Caitlin Cary was raised with her half-brothers, Brian, Craig, and Keith Thomas, in East Cleveland and Cleveland Heights. She began playing the violin at age six. She attended the College of Wooster in Ohio. She joined the band Whiskeytown in 1994, as a graduate student at North Carolina State University.
Cary released her first solo EP, Waltzie, in 2000. She has since released two full-length solo albums and an album of duets with Thad Cockrell. Cary has collaborated on albums with such artists as Tres Chicas, Alejandro Escovedo, Kenny Roby, and Greg Hawks and The Tremblers.
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